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    Effect of charge ordering on crossplane thermal conductivity in correlated perovskite oxide superlattices

    P. Thiessen1,*, V. Roddatis1, F. Rieger1, A. Belenchuk2, M. Keunecke3, V. Moshnyaga3, and Ch. Jooss1

    • 1Institute of Materials Physics, University of Göttingen, D-37077 Göttingen, Germany
    • 2IIEN, Academy of Sciences of Moldova, MD2028 Chisinau, Moldova
    • 3First Physical Institute, University of Göttingen, D-37077 Göttingen, Germany

    • *Present address: Institute of Physics, University of Hamburg, D-22761 Hamburg, Germany.

    Phys. Rev. B 98, 195114 – Published 13 November, 2018

    DOI: https://doi.org/10.1103/PhysRevB.98.195114

    Abstract

    Lattice thermal conductivity is a sensitive probe of distortions of the translational invariance of crystalline materials. Crossplane thermal conductivity, κ(T), was studied by the 3ω technique in superlattices, comprising orthorhombic charge/orbital ordered manganite Pr0.7Ca0.3MnO3 and cubic SrTiO3. The manganite/titanite superlattices show a peak in κ(T) just above the charge order transition temperature TCO∼240K with a pronounced thermal hysteresis. This ordering peak in κ(T) is successively suppressed with decreasing layer thickness. Our results demonstrate a minor effect of the interface density on κ, primarily visible below TCO. In contrast, much higher changes in κ(T) evolve close to TCO, due to interface-induced effects on charge and orbital ordering. Our results suggest that the ordering peak in κ(T) is a result of lattice softening above the phase transition which is modified by thickness-dependent misfit strain.

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